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Third harmonic generation in a Quantum Cascade laser with monolithically integrated resonant optical nonlinearity

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Abstract

We present third harmonic generation from an InGaAs/AlInAs Quantum Cascade laser based on a three-well diagonal transition active region with an integrated third-order nonlinear oscillator. The device displays pump radiation at λ~11.1 µm and third order nonlinear light generation at λ~3.7 µm as well as second harmonic generation at λ~5.4 µm.

©2004 Optical Society of America

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Figures (2)

Fig. 1.
Fig. 1. Conduction band energy diagram for one active region between two injector regions. The significant energy levels inside the active region are labeled 1 to 5. The thicknesses in nanometers of the InGaAs QW’s and AlInAs barriers of one period of injector and active region are from right to left: 3.7/2.1/3.0/2.1/3.5/2.1/3.4/3.6/3.1/1.2/6.4/1.3/4.7/2.6, the barriers are indicated in bold font and the underlined layers are doped to nSi=2.5×1016 cm-3. The yellow bars indicate the levels involved in THG; the red bars and arrow indicates the laser transition.
Fig. 2.
Fig. 2. Emission spectra of a QC laser with integrated third-order nonlinear oscillator in the active region. Part (A) shows the spectrum of the fundamental light emission at a wavelength of 11.1 µm. The spectrum was taken with a MCT detector. Part (B) shows the SHG and THG light emission from the same device. The SHG and THG are at wavelengths of 5.4 µm and 3.7 µm, respectively. The spectra were taken with an InSb detector.

Equations (6)

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P ( 3 ω ) = e N e z 25 σ 52
i e 4 z 23 z 34 z 45 z 25 N e E z 3 ( ω ) 3 Γ 52 ( 1 Γ 42 ( n 3 n 4 Γ 43 + n 3 n 2 Γ 32 ) 1 Γ 53 ( n 4 n 5 Γ 54 n 3 n 4 Γ 43 ) )
χ ( 3 ) χ ( 2 ) e z 52 γ 52 10 3 .
W 3 2 10 π 6 Σ W 1 3 [ 1 + e 2 α 3 L 2 e α 3 L cos ( Δ k L ) ] · ( 1 R 3 ) μ 1 3 μ 3 c 2 λ 3 2 ( Δ k 2 + α 3 2 ) ( 1 R 1 ) 3 ,
Σ =
μ 1 6 μ 3 2 ( χ ( 3 ) ( x , z ) 1 ε ω 3 H ω 3 H 3 ω dxdz 2 1 ε 3 ω H 3 ω 2 dxdz ) ( ( H 3 ω 2 dxdz ) 2 ( 1 ε ω H ω 2 dxdz ) 3 )
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